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Performance of an ANAMMOX reactor treating wastewater generated by antibiotic and starch production processes

Hong YAO, Hao LIU, Yongmiao HE, Shujun ZHANG, Peizhe SUN, Chinghua HUANG

《环境科学与工程前沿(英文)》 2012年 第6卷 第6期   页码 875-883 doi: 10.1007/s11783-012-0459-y

摘要: A pilot-scale anaerobic ammonia oxidation (ANAMMOX) reactor was used to treat mixed wastewater resulting from a chlortetracycline and starch production process. The results, collected over the course of 272 days, show that the ratio of influent ammonium to nitrite, pH, and temperature can all affect the efficiency of nitrogen removal. The ratio of influent ammonium to nitrite was maintained at about 1:1 at a concentration below 200 mg·L for both influent ammonium and nitrite. The total nitrogen (TN) loading rate was 0.15–0.30 kgN·m ·d , pH remained at 7.8–8.5, and temperature was recorded at 33±1°C. The rate of removal of ammonia, nitrite, and TN were over 90%, 90%, and 80%, and the effluent ammonium, nitrite and TN concentrations were below 50, 30, and 100 mg·L .

关键词: anaerobic ammonia oxidation     antibiotic and starch production     ratio of ammonia to nitrite     total nitrogen    

Enhancement on the ammonia oxidation capacity of ammonia-oxidizing archaeon originated from wastewater

《环境科学与工程前沿(英文)》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1375-1

摘要:

• AOA’s ammonia oxidizing capacity was enhanced under moderate magnetic field.

关键词: Ammonia-oxidizing archaeon     Ammonia oxidation     Magnetic field     Magnetotaxis     Heredity    

Electricity-driven ammonia oxidation and acetate production in microbial electrosynthesis systems

《环境科学与工程前沿(英文)》 2022年 第16卷 第4期 doi: 10.1007/s11783-021-1476-5

摘要:

• MES was constructed for simultaneous ammonia removal and acetate production.

关键词: Biocathode     Carbon dioxide     Electrochemical oxidation     Graphite anode     Boron-doped diamond    

Platinum on nitrogen doped graphene and tungsten carbide supports for ammonia electro-oxidation reaction

《化学科学与工程前沿(英文)》 2022年 第16卷 第6期   页码 930-938 doi: 10.1007/s11705-021-2130-2

摘要: Ammonia electrooxidation reaction involving multistep electron-proton transfer is a significant reaction for fuel cells, hydrogen production and understanding nitrogen cycle. Platinum has been established as the best electrocatalyst for ammonia oxidation in aqueous alkaline media. In this study, Pt/nitrogen-doped graphene (NDG) and Pt/tungsten monocarbide (WC)/NDG are synthesized by a wet chemistry method and their ammonia oxidation activities are compared to commercial Pt/C. Pt/NDG exhibits a specific activity of 0.472 mA∙cm–2, which is 44% higher than commercial Pt/C, thus establishing NDG as a more effective support than carbon black. Moreover, it is demonstrated that WC as a support also impacts the activity with further 30% increase in comparison to NDG. Surface modification with Ir resulted in the best electrocatalytic activity with Pt-Ir/WC/NDG having almost thrice the current density of commercial Pt/C. This work adds insights regarding the role of NDG and WC as efficient supports along with significant impact of Ir surface modification.

关键词: Ammonia electro-oxidation reaction     electrocatalyst supports     platinum     nitrogen doped graphene     tungsten carbide    

The combined effects of biomass and temperature on maximum specific ammonia oxidation rate in domestic

《环境科学与工程前沿(英文)》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1411-9

摘要:

• Actual SAORs was determined using MLVSS and temperature.

关键词: Specific ammonia oxidation rate     Sequencing batch reactor     Biomass     Temperature coefficient     Model simulation    

Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

《环境科学与工程前沿(英文)》 2014年 第8卷 第4期   页码 598-606 doi: 10.1007/s11783-013-0576-2

摘要: A novel hybrid anaerobic-contact oxidation biofilm baffled reactor (HAOBR) was developed to simultaneously remove nitrogenous and carbonaceous organic pollutants from decentralized molasses wastewater in the study. The study was based on the inoculation of anaerobic granule sludge in anaerobic compartments and the installation of combination filler in aerobic compartments. The performance of reactor system was studied regarding the hydraulic retention time (HRT), microbial characteristics and the gas water ratio (GWR). When the HRT was 24h and the GWR was 20:1, total ammonia and chemical oxygen demand (COD) of the effluent were reduced by 99% and 91.8%, respectively. The reactor performed stably for treating decentralized molasses wastewater. The good performance of the reactor can be attributed to the high resistance of COD and hydraulic shock loads. In addition, the high solid retention time of contact oxidation biofilm contributed to stable performance of the reactor.

关键词: combination filler     contact oxidation biofilm     food wastewater     anaerobic baffled reactor    

Comparison of different valent iron on anaerobic sludge digestion: Focusing on oxidation reduction potential

《环境科学与工程前沿(英文)》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1514-3

摘要:

• ORP value from −278.71 to −379.80 mV showed indiscernible effects on methane yield.

关键词: Enhanced anaerobic sludge digestion     Different iron valence     Oxidation reduction potential     Dissolved organic nitrogen     Microbial community    

ROOT EXUDATES FROM CANOLA EXHIBIT BIOLOGICAL NITRIFICATION INHIBITION AND ARE EFFECTIVE IN INHIBITING AMMONIAOXIDATION IN SOIL

《农业科学与工程前沿(英文)》 2022年 第9卷 第2期   页码 177-186 doi: 10.15302/J-FASE-2021421

摘要:

A range of plant species produce root exudates that inhibit ammonia-oxidizing microorganisms. This biological nitrification inhibition (BNI) capacity can decrease N loss and increase N uptake from the rhizosphere. This study sought evidence for the existence and magnitude of BNI capacity in canola ( Brassica napus). Seedlings of three canola cultivars, Brachiaria humidicola(BNI positive) and wheat ( Triticum aestivum) were grown in a hydroponic system. Root exudates were collected and their inhibition of the ammonia oxidizing bacterium, Nitrosospira multiformis, was tested. Subsequent pot experiments were used to test the inhibition of native nitrifying communities in soil. Root exudates from canola significantly reduced nitrification rates of both N. multiformis cultures and native soil microbial communities. The level of nitrification inhibition across the three cultivars was similar to the well-studied high-BNI species B. humidicola. BNI capacity of canola may have implications for the N dynamics in farming systems and the N uptake efficiency of crops in rotational farming systems. By reducing nitrification rates canola crops may decrease N losses, increase plant N uptake and encourage microbial N immobilization and subsequently increase the pool of organic N that is available for mineralization during the following cereal crops.

关键词: ammonia oxidizing microorganisms / biological nitrification inhibition / farming rotations / nitrogen cycling / nitrogen use efficiency    

Anoxic phosphorus removal in a pilot scale anaerobic-anoxic oxidation ditch process

Hongxun HOU, Shuying WANG, Yongzhen PENG, Zhiguo YUAN, Fangfang YIN, Wang GAN

《环境科学与工程前沿(英文)》 2009年 第3卷 第1期   页码 106-111 doi: 10.1007/s11783-009-0005-8

摘要: The anaerobic-anoxic oxidation ditch (A /O OD) process is popularly used to eliminate nutrients from domestic wastewater. In order to identify the existence of denitrifying phosphorus removing bacteria (DPB), evaluate the contribution of DPB to biological nutrient removal, and enhance the denitrifying phosphorus removal in the A /O OD process, a pilot-scale A /O OD plant (375 L) was conducted. At the same time batch tests using sequence batch reactors (12 L and 4 L) were operated to reveal the significance of anoxic phosphorus removal. The results indicated that: The average removal efficiency of COD, , , and TN were 88.2%, 92.6%, 87.8%, and 73.1%, respectively, when the steady state of the pilot-scale A /O OD plant was reached during 31-73 d, demonstrating a good denitrifying phosphorus removal performance. Phosphorus uptake took place in the anoxic zone by poly-phosphorus accumulating organisms could be used as electron receptors in denitrifying phosphorus removal, and the phosphorus uptake rate with as the electron receptor was higher than that with when the initial concentration of either or was 40 mg/L.

关键词: wastewater treatment     anaerobic-anoxic (A2/O)     oxidation ditch (OD)     biological phosphorus removal     denitrifying phosphorus removal    

Influence of influent on anaerobic ammonium oxidation in an Expanded Granular Sludge Bed-Biological Aerated

Daijun ZHANG, Cui BAI, Ting TANG, Qing YANG

《环境科学与工程前沿(英文)》 2011年 第5卷 第2期   页码 291-297 doi: 10.1007/s11783-010-0270-6

摘要: Shortcut nitrification-denitrification, anaerobic ammonium oxidation (ANAMMOX), and methanogenesis have been successfully coupled in an Expanded Granular Sludge Bed-Biological Aerated Filter (EGSB-BAF) integrated system. As fed different synthetic wastewater with chemical oxygen demand (COD) of 300–1200 mg·L and of 30–120 mg·L at the outer recycle ratio of 200%, the influence of influent on ANAMMOX in the integrated system was investigated in this paper. The experimental results showed that higher COD concentration caused an increase in denitrification and methanogenesis but a decrease in ANAMMOX; however, when an influent with the low concentration of COD was used, the opposite changes could be observed. Higher influent concentration favored ANAMMOX when the COD concentration of influent was fixed. Therefore, low ratio would decrease competition for nitrite between ANAMMOX and denitrification, which was favorable for reducing the negative effect of organic COD on ANAMMOX. The good performance of the integrated system indicated that the bacterial community of denitrification, ANAMMOX, and methanogenesis could be dynamically maintained in the sludge of EGSB reactor for a certain range of influent.

关键词: Expanded Granular Sludge Bed-Biological Aerated Filter (EGSB-BAF) integrated system     the influence of influent     anaerobic ammonium oxidation (ANAMMOX)     shortcut nitrification-denitrification     methano-genesis    

Overlooked nitrogen-cycling microorganisms in biological wastewater treatment

《环境科学与工程前沿(英文)》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1426-2

摘要:

• AOA and comammox bacteria can be more abundant and active than AOB/NOB at WWTPs.

关键词: Ammonia oxidizing archaea (AOA)     Complete ammonia oxidizing (comammox) bacteria     Dissimilatory nitrate reduction to ammonium (DNRA) bacteria     Nitrate/nitrite-dependent anaerobic methane oxidizing (NOx-DAMO) microorganisms     Engineering application    

Influencing mechanism of high solid concentration on anaerobic mono-digestion of sewage sludge without

Yuyao ZHANG,Huan LI,Can LIU,Yingchao CHENG

《环境科学与工程前沿(英文)》 2015年 第9卷 第6期   页码 1108-1116 doi: 10.1007/s11783-015-0806-x

摘要: High-solids anaerobic digestion of sewage sludge was a promising process, but high solid concentration negatively influenced methane production. The influencing mechanism was systematically analyzed in this study through a series of static anaerobic digestion experiments at total solids (TS) contents of 3%–15%. The results showed that TS 6% was the boundary between low-solids and high-solids anaerobic digestion, and the accumulative methane yield decreased exponentially when TS increased from 6% to 15%. The performance of anaerobic digestion was directly determined by the efficiency of mass transfer, and the relation between methane yield and sludge diffusive coefficients was well described by a power function. Thus, the increasing TS resulted in an exponential increase in sludge viscosity but an exponential decrease in diffusive coefficient. The blocked mass transfer led to the accumulation of volatile fatty acids (VFAs) and free ammonia. Acetic metabolism was the main process, whereas butyric and propionic metabolisms occurred at the initial stage of high-solids anaerobic digestion. The concentration of VFAs reached the maximum at the initial stage, which were still lower than the threshold influencing methanogens. The concentration of free ammonia increased gradually, and the methanogenesis was inhibited when free ammonia nitrogen exceeded 50 mg·L . Consequently, the deterioration of high-solids anaerobic digestion was related to the blocked mass transfer and the resulting ammonia accumulation.

关键词: anaerobic digestion     methane     sewage sludge     volatile fatty acids     free ammonia    

Anaerobic ammonia oxidizing bacteria: ecological distribution, metabolism, and microbial interactions

Dawen Gao, Xiaolong Wang, Hong Liang, Qihang Wei, Yuan Dou, Longwei Li

《环境科学与工程前沿(英文)》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1035-x

摘要: Anammox (ANaerobic AMMonia OXidation) is a newly discovered pathway in the nitrogen cycle. This discovery has increased our knowledge of the global nitrogen cycle and triggered intense interest for anammox-based applications. Anammox bacteria are almost ubiquitous in the suboxic zones of almost all types of natural ecosystems and contribute significant to the global total nitrogen loss. In this paper, their ecological distributions and contributions to the nitrogen loss in marine, wetland, terrestrial ecosystems, and even extreme environments were reviewed. The unique metabolic mechanism of anammox bacteria was well described, including the particular cellular structures and genome compositions, which indicate the special evolutionary status of anammox bacteria. Finally, the ecological interactions among anammox bacteria and other organisms were discussed based on substrate availability and spatial organizations. This review attempts to summarize the fundamental understanding of anammox, provide an up-to-date summary of the knowledge of the overall anammox status, and propose future prospects for anammox. Based on novel findings, the metagenome has become a powerful tool for the genomic analysis of communities containing anammox bacteria; the metabolic diversity and biogeochemistry in the global nitrogen budget require more comprehensive studies.

关键词: Anammox     Metabolism     Metagenome     Ecological distribution     Microbial interactions    

Occurrence and behavior of pharmaceuticals in sewage treatment plants in eastern China

Juan DU,Yu FAN,Xin QIAN

《环境科学与工程前沿(英文)》 2015年 第9卷 第4期   页码 725-730 doi: 10.1007/s11783-014-0661-1

摘要: The occurrence and removal efficiency of seven pharmaceuticals (norfloxacin, trimethoprim, roxithromycin, sulfamethoxazole, ibuprofen, diclofenac and carbamazepine) were determined in three sewage treatment plants (STPs) with anaerobic/anoxic/oxic, anoxic/oxic and oxidation ditches processes in Xuzhou City, Eastern China. The results showed that seven pharmaceuticals were detected in the influent samples with concentrations ranging from 93 to 2540 ng·L . The removal of these substances among the three different STPs varied from 36 to 84%, with the highest performance obtained by the wastewater treatment works with tertiary treatment (sand filtration). Most of the compounds were removed effectively during biologic treatment while sand filtration treatment also made a contribution to the total elimination of most pharmaceuticals. The efficiency comparison of the three sewage treatment processes showed that the STP which employed anaerobic/anoxic/oxic was more effective to remove pharmaceuticals than the oxidation ditches and anoxic/oxic.

关键词: pharmaceutical     anaerobic/anoxic/oxic     oxidation ditch     anoxic/oxic     removal efficiency    

The main anammox-based processes, the involved microbes and the novel process concept from the application perspective

《环境科学与工程前沿(英文)》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1487-1

摘要:

• The PNA, denitratation/anammox, and DAMO/anammox process are reviewed together.

关键词: Anammox     Nitritation     Denitratation     Denitrifying anaerobic methane oxidation     Mainstream wastewater    

标题 作者 时间 类型 操作

Performance of an ANAMMOX reactor treating wastewater generated by antibiotic and starch production processes

Hong YAO, Hao LIU, Yongmiao HE, Shujun ZHANG, Peizhe SUN, Chinghua HUANG

期刊论文

Enhancement on the ammonia oxidation capacity of ammonia-oxidizing archaeon originated from wastewater

期刊论文

Electricity-driven ammonia oxidation and acetate production in microbial electrosynthesis systems

期刊论文

Platinum on nitrogen doped graphene and tungsten carbide supports for ammonia electro-oxidation reaction

期刊论文

The combined effects of biomass and temperature on maximum specific ammonia oxidation rate in domestic

期刊论文

Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

期刊论文

Comparison of different valent iron on anaerobic sludge digestion: Focusing on oxidation reduction potential

期刊论文

ROOT EXUDATES FROM CANOLA EXHIBIT BIOLOGICAL NITRIFICATION INHIBITION AND ARE EFFECTIVE IN INHIBITING AMMONIAOXIDATION IN SOIL

期刊论文

Anoxic phosphorus removal in a pilot scale anaerobic-anoxic oxidation ditch process

Hongxun HOU, Shuying WANG, Yongzhen PENG, Zhiguo YUAN, Fangfang YIN, Wang GAN

期刊论文

Influence of influent on anaerobic ammonium oxidation in an Expanded Granular Sludge Bed-Biological Aerated

Daijun ZHANG, Cui BAI, Ting TANG, Qing YANG

期刊论文

Overlooked nitrogen-cycling microorganisms in biological wastewater treatment

期刊论文

Influencing mechanism of high solid concentration on anaerobic mono-digestion of sewage sludge without

Yuyao ZHANG,Huan LI,Can LIU,Yingchao CHENG

期刊论文

Anaerobic ammonia oxidizing bacteria: ecological distribution, metabolism, and microbial interactions

Dawen Gao, Xiaolong Wang, Hong Liang, Qihang Wei, Yuan Dou, Longwei Li

期刊论文

Occurrence and behavior of pharmaceuticals in sewage treatment plants in eastern China

Juan DU,Yu FAN,Xin QIAN

期刊论文

The main anammox-based processes, the involved microbes and the novel process concept from the application perspective

期刊论文